Investigation of non-thermal atmospheric plasma for the degradation of avermectin solution
文献类型： 外文期刊
作者： LV, Yue 1 ; ZOU, Liang 1 ; LI, Huidong 2 ; CEHN, Zilei 2 ; WANG, Xiaolong 1 ; SUN, Ying 1 ; FANG, Liping 2 ; ZHAO, Tong 1 ;
作者机构： 1.Shandong Univ, Sch Elect Engn, Jinan 250061, Peoples R China
2.Shandong Acad Agr Sci, Inst Agr Qual Stand & Testing Technol, Jinan 250061, Peoples R China
关键词： non-thermal atmospheric plasma; pesticide degradation; avermectins; molecular dynamics simulation
期刊名称：PLASMA SCIENCE & TECHNOLOGY （ 影响因子：1.358； 五年影响因子：1.157 ）
ISSN： 1009-0630
年卷期： 2021 年 23 卷 5 期
页码：
收录情况： SCI
摘要： Increasing concern with regard to food safety in the presence of pesticide residues (PRs) on the surface of agricultural products has resulted in the rapid development of practical degrading technologies for corresponding PRs. In this paper, an unconventional method of degrading pesticides, non-thermal atmospheric plasma (NTAP), was proposed to degrade the avermectin (AVM) in aqueous solution. Optical emission spectroscopy shows that NTAP, consisting of filamentary streamers, contains a variety of reactive oxygen species (ROS) that may interact with AVM. The high-performance liquid chromatography (HPLC)-MS/MS results indicate that the efficiency of AVM degradation seriously depends on multiple operation parameters of the NTAP, including the applied voltage, treatment time and gas flow rate. The maximum degradation rate of AVM was observed to be 97.47% after 240 s exposure under NTAP with an applied voltage of 18 kV and gas flow rate of 1 l min(-1). Molecular dynamics simulation based on a reactive force field for the interaction between O (ground state atomic oxygen) and AVM was performed to analyze the underpinning mechanisms. The simulation result shows the possible pathways of the NTAP-generated O degrading AVM by destroying the glycosyl group or fracturing the ester group.
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