Release and Degradation Mechanism of Modified Polyvinyl Alcohol-Based Double-Layer Coated Controlled-Release Phosphate Fertilizer
文献类型： 外文期刊
作者： Sun, Teng 1 ; Zhan, Dekang 1 ; Wang, Xiangzhu 1 ; Guo, Qingjie 1 ; Wu, Mingzhou 2 ; Shen, Pu 3 ; Wu, Man 1 ;
作者机构： 1.Qingdao Univ Sci & Technol, Lab Green & Smart Chem Engn Univ Shandong, Coll Chem Engn, Qingdao 266042, Peoples R China
2.Shenzhen Technol Univ, Coll Hlth Sci & Environm Engn, Shenzhen 518118, Peoples R China
3.Shandong Acad Agr Sci, Minist Agr & Rural Affairs, Shandong Peanut Res Inst, Key Lab Peanut Biol Genet & Breeding, 126 Wannianquan Rd, Qingdao 266100, Peoples R China
关键词： controlled release; phosphate fertilizers; biochar doping; biodegradability; double-layer film; polyvinyl alcohol
期刊名称：POLYMERS （ 影响因子：5.0； 五年影响因子：5.0 ）
ISSN：
年卷期： 2024 年 16 卷 8 期
页码：
收录情况： SCI
摘要： This study aims to improve the slow-release performance of a film material for a controlled-release fertilizer (CRF) while enhancing its biodegradability. A water-based biodegradable polymer material doped with biochar (BC) was prepared from modified polyvinyl alcohol (PVA) with polyvinylpyrrolidone (PVP) and chitosan (CTS), hereinafter referred to as PVA/PVP-CTSaBCb. An environmentally friendly novel controlled-release phosphate fertilizer (CRPF) was developed using PVA/PVP-CTS8%BC7% as the film. The effect of the PVA/PVP-CTS8%BC7% coating on the service life of the CRPF was investigated. The film was characterized via stress-strain testing, SEM, FTIR, XRD, and TGA analyses. The addition of the CTS modifier increased the stress of PVA/PVP-CTS8% by 7.6% compared with that of PVA/PVP owing to the decrease in the crystallinity of PVP/PVP-CTS8%. The hydrophilic -OH groups were reduced due to the mixing of CTS and PVA/PVP. Meanwhile, the water resistance of the PVA/PVP-CTS8%BC7% was improved. And the controlled-release service life of the CRPF was prolonged. Moreover, the addition of BC increased the crystallinity of the PVA/PVP-CTS8% by 10%, reduced the fracture elongation of the material, and further improved the biodegradability of the PVA/PVP-CTS8%BC7%. When the amount of BC added was 7%, the phosphorus release rate of the CRPF was 30% on the 28th day. Moreover, the degradation rate of the PVA/PVP-CTS8%BC7% polymer film was 35% after 120 days. This study provides basic data for applying water-based degradable polymer materials in CRFs.
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